I see this pretty often actually:

Adding a new article via the Safari extension, Zotero will hang, with the fans on my MBP going like mad. After a few minutes I give up and kill it. Then a restart gives the same result.

I'm in the third iteration right now and it's finally calmed down and become responsive after a few minutes. The .hang file in the OS X logs says this:

Command: zotero-bin
Path: /Applications/Zotero.app/Contents/MacOS/zotero-bin
Process: zotero-bin [12506]
Path: /Applications/Zotero.app/Contents/MacOS/zotero-bin
0x100000000 - 0x100002ff7 zotero-bin <156CCD6D-AEB4-357A-AD9D-728E145BABCA> /Applications/Zotero.app/Contents/MacOS/zotero-bin
0x100400000 - 0x100672ff7 libnss3.dylib (1) <40D15904-530A-3FE6-97A7-6FAC8C2F96C6> /Applications/Zotero.app/Contents/MacOS/libnss3.dylib
0x101000000 - 0x105327fc7 XUL (1) <71752593-29A7-3DCE-A03F-6344268E2351> /Applications/Zotero.app/Contents/MacOS/XUL
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